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Abstract Most stars are born in stellar clusters, and their protoplanetary disks, which are the birthplaces of planets, can, therefore, be affected by the radiation of nearby massive stars. However, little is known about the chemistry of externally irradiated disks, including whether or not their properties are similar to the so-far better-studied isolated disks. Motivated by this question, we present ALMA Band 6 observations of two irradiated Class II protoplanetary disks in the outskirts of the Orion Nebula Cluster to explore the chemical composition of disks exposed to (external) far-ultraviolet (FUV) radiation fields: the 216-0939 disk and the binary system 253-1536A/B, which are exposed to radiation fields of 10²–10³times the average interstellar radiation field. We detect lines from CO isotopologues, HCN, H₂CO, and C₂H toward both protoplanetary disks. Based on the observed disk-integrated line fluxes and flux ratios, we do not find significant differences between isolated and irradiated disks. The observed differences seem to be more closely related to the different stellar masses than to the external radiation field. This suggests that these disks are far enough away from the massive Trapezium stars, that their chemistry is no longer affected by external FUV radiation. Additional observations toward lower-mass disks and disks closer to the massive Trapezium stars are required to elucidate the level of external radiation required to make an impact on the chemistry of planet formation in different kinds of disks. 

Abstract H₂CO is a small organic molecule widely detected in protoplanetary disks. As a precursor to grain-surface formation of CH₃OH, H₂CO is considered an important precursor of O-bearing organic molecules that are locked in ices. Still, since gas-phase reactions can also form H₂CO, there remains an open question on the channels by which organics form in disks, and how much the grain versus the gas pathways impact the overall organic reservoir. We present spectrally and spatially resolved Atacama Large Millimeter/submillimeter Array observations of several ortho- and para-H₂CO transitions toward the bright protoplanetary disk around the Herbig Ae star HD 163296. We derive column density, excitation temperature, and ortho-to-para ratio (OPR) radial profiles for H₂CO, as well as disk-averaged values ofN_T∼ 4 × 10¹²cm⁻²,T_ex∼ 20 K, and OPR ∼ 2.7, respectively. We empirically determine the vertical structure of the emission, finding vertical heights ofz/r∼ 0.1. From the profiles, we find a relatively constant OPR ∼ 2.7 with radius, but still consistent with 3.0 among the uncertainties, a secondary increase ofN_Tin the outer disk, and lowT_exvalues that decrease with disk radius. Our resulting radial, vertical, and OPR constraints suggest an increased UV penetration beyond the dust millimeter edge, consistent with an icy origin but also with cold gas-phase chemistry. This Herbig disk contrasts previous results for the T Tauri disk, TW Hya, which had a larger contribution from cold gas-phase chemistry. More observations of other sources are needed to disentangle the dominant formation pathway of H₂CO in protoplanetary disks.